I'd say the 2 best were TMO and IB. Those guys were on equal footing and traded the top spot back and forth for a while.
Rampage after their merger/creation along with the formation of Forsaken splitting TMO members gave Rampage a numbers advantage for a large portion of early Velious. When guilds started working together to even those numbers up or surpass them Rampage struggled.
Awakened and Aftermath are too early to tell really. They haven't had the lifespan of the other guilds mentioned yet.
Twist my arm...IB 1rst with TMO in a close 2nd if we are talking last 3 years. TMO did outlast IB though and killed more of the Top mob in that era (PD). But the kill count would probably slightly favor IB overall over the span they competed against each other.
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