Neriak, Grobb, and Felwithe guards are the most popular to hunt imo, just from experience on blue. Kaladim guards has fans as well. They're also some of the best sources of level 40 npcs to take you to level 55.
Neriak cleric guild (with pulling inner faction guards from the area around the library and rogue guilds) will take you to level 55 quickly in a Mage/Cleric duo, and I'd presume its just as quick with necro/dps.
But realistically average players won't get to ride on spots like that as they'll be locked down by guilds who won't share, as such spots are a safer bet than FFA bard power leveling in BW / DL. However people that have done the Live classic progression seem to have plenty of experience with this Kunark rush already so maybe there are some spots in kunark that blow guards out of the water. I'm sure some masochist will chime in with Kedge purely for its zem, but if I were you I'd aim for level 51 and a OT gate hammer + CoS then try for guard leveling (if you're hellbent on it) after the rush or at odd hours.
Good luck!
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