Just charm animals on the druid and have your sister help out when things are going sideways. It'll be far more efficient than trying to heal / DS / manage the paladin. You'll still be doing the heavy lifting, but it won't quite be the show-stealer that is enchanter (or charming necro for that matter).
Oasis crocs are great to cut your teeth on the method / strategy. From there, you can bounce around the outdoor zones until you get high enough for Cazic Thule. Its one of the highest ZEMs in the game, and you'll want to charm the crocs there until they basically green out. Not sure what level that gets you to, but it will be insane XP.
Maybe after / as a break from CT you could consider doing Overthere and funneling all the braid turn-ins to the paladin for a free OT hammer (bind at HH on the druid and no matter what your sister goes off and does by herself you guys can reunite quickly). In your late 40s you can do Bats n Bugs in SolB, Emerald Jungle has some gorillas, then once you get Call of Karana at 52 you can head over to Chardok for a few levels. You'll probably do 54/55 to 60 exclusively in Bear Pits way down in the bottom of Permafrost. Heck, even Kedge is an option if you want a challenge.
Having the pally there to stun / pick up broken charm pets will essentially take all the risk out of charm solo. Additionally, you don't have to worry about the charmed pet eating 50% of the XP in a duo. Just haste / DS the pet and let it tank until it gets low. Break the pet w/ invis vs animals (dispel it if its hasted / DS), and you and the pally finish it off for full xp. The paladin should only be taking damage when helping you with charm breaks, pulls gone sideways, or finishing off mobs if there is no other animal around to charm and do it for you.
That being said...you can always /who all and add a bard, enc, or shaman and trio with a dedicated slower. This will allow you to sit back and heal / CC and let your sister do some real tanking for a change (bonus points if you still continue to maintain a charm pet too)...and let you go explore some other awesome dungeons (early Permafrost, Splitpaw, Guk, etc).
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